Effects of sources and meteorology on particulate matter in the Western Mediterranean Basin: An overview of the DAURE campaign

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Effects of sources and meteorology on particulate matter in the Western Mediterranean Basin : An overview of the DAURE campaign. / Pandolfi, M.; Querol, X.; Alastuey, A.; Jimenez, J. L.; Jorba, O.; Day, D.; Ortega, A.; Cubison, M. J.; Comerón, A.; Sicard, M.; Mohr, C.; Prévôt, A. S. H.; Minguillón, M. C.; Pey, J.; Baldasano, J. M.; Burkhart, J. F.; Seco, R.; Peñuelas, J.; Van Drooge, B. L.; Artiñano, B.; Di Marco, C.; Nemitz, E.; Schallhart, S.; Metzger, A.; Hansel, A.; Lorente, J.; Ng, S.; Jayne, J.; Szidat, S.

I: Journal of Geophysical Research: Atmospheres, Bind 119, Nr. 8, 2014, s. 4978-5010.

Publikation: Bidrag til tidsskrift › Tidsskriftartikel › Forskning › fagfællebedømt

Harvard

Pandolfi, M, Querol, X, Alastuey, A, Jimenez, JL, Jorba, O, Day, D, Ortega, A, Cubison, MJ, Comerón, A, Sicard, M, Mohr, C, Prévôt, ASH, Minguillón, MC, Pey, J, Baldasano, JM, Burkhart, JF, Seco, R, Peñuelas, J, Van Drooge, BL, Artiñano, B, Di Marco, C, Nemitz, E, Schallhart, S, Metzger, A, Hansel, A, Lorente, J, Ng, S, Jayne, J & Szidat, S 2014, 'Effects of sources and meteorology on particulate matter in the Western Mediterranean Basin: An overview of the DAURE campaign', Journal of Geophysical Research: Atmospheres, bind 119, nr. 8, s. 4978-5010. https://doi.org/10.1002/2013JD021079

APA

Pandolfi, M., Querol, X., Alastuey, A., Jimenez, J. L., Jorba, O., Day, D., Ortega, A., Cubison, M. J., Comerón, A., Sicard, M., Mohr, C., Prévôt, A. S. H., Minguillón, M. C., Pey, J., Baldasano, J. M., Burkhart, J. F., Seco, R., Peñuelas, J., Van Drooge, B. L., ... Szidat, S. (2014). Effects of sources and meteorology on particulate matter in the Western Mediterranean Basin: An overview of the DAURE campaign. Journal of Geophysical Research: Atmospheres, 119(8), 4978-5010. https://doi.org/10.1002/2013JD021079

Vancouver

Pandolfi M, Querol X, Alastuey A, Jimenez JL, Jorba O, Day D o.a. Effects of sources and meteorology on particulate matter in the Western Mediterranean Basin: An overview of the DAURE campaign. Journal of Geophysical Research: Atmospheres. 2014;119(8):4978-5010. https://doi.org/10.1002/2013JD021079

Author

Pandolfi, M. ; Querol, X. ; Alastuey, A. ; Jimenez, J. L. ; Jorba, O. ; Day, D. ; Ortega, A. ; Cubison, M. J. ; Comerón, A. ; Sicard, M. ; Mohr, C. ; Prévôt, A. S. H. ; Minguillón, M. C. ; Pey, J. ; Baldasano, J. M. ; Burkhart, J. F. ; Seco, R. ; Peñuelas, J. ; Van Drooge, B. L. ; Artiñano, B. ; Di Marco, C. ; Nemitz, E. ; Schallhart, S. ; Metzger, A. ; Hansel, A. ; Lorente, J. ; Ng, S. ; Jayne, J. ; Szidat, S. / Effects of sources and meteorology on particulate matter in the Western Mediterranean Basin : An overview of the DAURE campaign. I: Journal of Geophysical Research: Atmospheres. 2014 ; Bind 119, Nr. 8. s. 4978-5010.

Bibtex

@article{c76eb9ca569945049d978c8652a178cc,
title = "Effects of sources and meteorology on particulate matter in the Western Mediterranean Basin: An overview of the DAURE campaign",
abstract = "DAURE (Determination of the Sources of Atmospheric Aerosols in Urban and Rural Environments in the Western Mediterranean) was a multidisciplinary international field campaign aimed at investigating the sources and meteorological controls of particulate matter in the Western Mediterranean Basin (WMB). Measurements were simultaneously performed at an urban-coastal (Barcelona, BCN) and a rural-elevated (Montseny,MSY) site pair in NE Spain during winter and summer. State-of-the-artmethods such as 14C analysis, proton-transfer reaction mass spectrometry, and high-resolution aerosol mass spectrometry were applied for the first time in the WMB as part of DAURE. WMB regional pollution episodes were associated with high concentrations of inorganic and organic species formed during the transport to inland areas and built up at regional scales. Winter pollutants accumulation depended on the degree of regional stagnation of an air mass under anticyclonic conditions and the planetary boundary layer height. In summer, regional recirculation and biogenic secondary organic aerosols (SOA) formation mainly determined the regional pollutant concentrations. The contribution from fossil sources to organic carbon (OC) and elemental carbon (EC) and hydrocarbon-like organic aerosol concentrations were higher at BCN compared with MSY due to traffic emissions. The relative contribution of nonfossil OC was higher at MSY especially in summer due to biogenic emissions. The fossil OC/EC ratio at MSY was twice the corresponding ratio at BCN indicating that a substantial fraction of fossil OC was due to fossil SOA. In winter, BCN cooking emissions were identified as an important source of modern carbon in primary organic aerosol.",
author = "M. Pandolfi and X. Querol and A. Alastuey and Jimenez, {J. L.} and O. Jorba and D. Day and A. Ortega and Cubison, {M. J.} and A. Comer{\'o}n and M. Sicard and C. Mohr and Pr{\'e}v{\^o}t, {A. S. H.} and Minguill{\'o}n, {M. C.} and J. Pey and Baldasano, {J. M.} and Burkhart, {J. F.} and R. Seco and J. Pe{\~n}uelas and {Van Drooge}, {B. L.} and B. Arti{\~n}ano and {Di Marco}, C. and E. Nemitz and S. Schallhart and A. Metzger and A. Hansel and J. Lorente and S. Ng and J. Jayne and S. Szidat",
year = "2014",
doi = "10.1002/2013JD021079",
language = "English",
volume = "119",
pages = "4978--5010",
journal = "Journal of Geophysical Research: Solid Earth",
issn = "0148-0227",
publisher = "American Geophysical Union",
number = "8",

}

RIS

TY - JOUR

T1 - Effects of sources and meteorology on particulate matter in the Western Mediterranean Basin

T2 - An overview of the DAURE campaign

AU - Pandolfi, M.

AU - Querol, X.

AU - Alastuey, A.

AU - Jimenez, J. L.

AU - Jorba, O.

AU - Day, D.

AU - Ortega, A.

AU - Cubison, M. J.

AU - Comerón, A.

AU - Sicard, M.

AU - Mohr, C.

AU - Prévôt, A. S. H.

AU - Minguillón, M. C.

AU - Pey, J.

AU - Baldasano, J. M.

AU - Burkhart, J. F.

AU - Seco, R.

AU - Peñuelas, J.

AU - Van Drooge, B. L.

AU - Artiñano, B.

AU - Di Marco, C.

AU - Nemitz, E.

AU - Schallhart, S.

AU - Metzger, A.

AU - Hansel, A.

AU - Lorente, J.

AU - Ng, S.

AU - Jayne, J.

AU - Szidat, S.

PY - 2014

Y1 - 2014

N2 - DAURE (Determination of the Sources of Atmospheric Aerosols in Urban and Rural Environments in the Western Mediterranean) was a multidisciplinary international field campaign aimed at investigating the sources and meteorological controls of particulate matter in the Western Mediterranean Basin (WMB). Measurements were simultaneously performed at an urban-coastal (Barcelona, BCN) and a rural-elevated (Montseny,MSY) site pair in NE Spain during winter and summer. State-of-the-artmethods such as 14C analysis, proton-transfer reaction mass spectrometry, and high-resolution aerosol mass spectrometry were applied for the first time in the WMB as part of DAURE. WMB regional pollution episodes were associated with high concentrations of inorganic and organic species formed during the transport to inland areas and built up at regional scales. Winter pollutants accumulation depended on the degree of regional stagnation of an air mass under anticyclonic conditions and the planetary boundary layer height. In summer, regional recirculation and biogenic secondary organic aerosols (SOA) formation mainly determined the regional pollutant concentrations. The contribution from fossil sources to organic carbon (OC) and elemental carbon (EC) and hydrocarbon-like organic aerosol concentrations were higher at BCN compared with MSY due to traffic emissions. The relative contribution of nonfossil OC was higher at MSY especially in summer due to biogenic emissions. The fossil OC/EC ratio at MSY was twice the corresponding ratio at BCN indicating that a substantial fraction of fossil OC was due to fossil SOA. In winter, BCN cooking emissions were identified as an important source of modern carbon in primary organic aerosol.

AB - DAURE (Determination of the Sources of Atmospheric Aerosols in Urban and Rural Environments in the Western Mediterranean) was a multidisciplinary international field campaign aimed at investigating the sources and meteorological controls of particulate matter in the Western Mediterranean Basin (WMB). Measurements were simultaneously performed at an urban-coastal (Barcelona, BCN) and a rural-elevated (Montseny,MSY) site pair in NE Spain during winter and summer. State-of-the-artmethods such as 14C analysis, proton-transfer reaction mass spectrometry, and high-resolution aerosol mass spectrometry were applied for the first time in the WMB as part of DAURE. WMB regional pollution episodes were associated with high concentrations of inorganic and organic species formed during the transport to inland areas and built up at regional scales. Winter pollutants accumulation depended on the degree of regional stagnation of an air mass under anticyclonic conditions and the planetary boundary layer height. In summer, regional recirculation and biogenic secondary organic aerosols (SOA) formation mainly determined the regional pollutant concentrations. The contribution from fossil sources to organic carbon (OC) and elemental carbon (EC) and hydrocarbon-like organic aerosol concentrations were higher at BCN compared with MSY due to traffic emissions. The relative contribution of nonfossil OC was higher at MSY especially in summer due to biogenic emissions. The fossil OC/EC ratio at MSY was twice the corresponding ratio at BCN indicating that a substantial fraction of fossil OC was due to fossil SOA. In winter, BCN cooking emissions were identified as an important source of modern carbon in primary organic aerosol.

U2 - 10.1002/2013JD021079

DO - 10.1002/2013JD021079

M3 - Journal article

AN - SCOPUS:84900523801

VL - 119

SP - 4978

EP - 5010

JO - Journal of Geophysical Research: Solid Earth

JF - Journal of Geophysical Research: Solid Earth

SN - 0148-0227

IS - 8

ER -

ID: 234281051